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Nonlinear Optical Resonances from Ballistic Electron Funnelling
Journal article   Peer reviewed

Nonlinear Optical Resonances from Ballistic Electron Funnelling

Hue T. B. Do, Gregory K. Ngirmang, Lin Wu and Michel Bosman
ACS nano, Vol.19(14), pp.14150-14160
15/04/2025
PMID: 40162829

Abstract

Chemistry Chemistry, Multidisciplinary Chemistry, Physical Materials Science Materials Science, Multidisciplinary Nanoscience & Nanotechnology Physical Sciences Science & Technology Science & Technology - Other Topics Technology
We introduce a new mechanism for second-harmonic generation through geometrically rectifying-funnelling-ballistic electrons in THz optical resonators. Our resonant rectifiers inherently act as second-order harmonic generators, rectifying currents without the presence of a potential barrier. Particle-in-cell simulations reveal that femtosecond electron-surface scattering plays a critical role in this process. We differentiate electron funnelling from nonlocal plasmonic drag and bulk Dirac anharmonicity, showing that funnelling can reduce the required field intensity for second-harmonic generation by 3-4 orders of magnitude. We provide design guidelines for generating funnelling-induced second-harmonic generation, including resonance mode matching and materials selection. This approach offers a practical pathway for low-field, geometrically tunable THz upconversion and rectification, operating from sub-10 THz to multiple tens of THz in graphene.

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