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The "inner and outer double-layer coating" constructs a three-dimensional electronic channel from the inside to the outside to improve the electrochemical performance of lithium iron phosphate
Journal article   Peer reviewed

The "inner and outer double-layer coating" constructs a three-dimensional electronic channel from the inside to the outside to improve the electrochemical performance of lithium iron phosphate

Chengyu Pan, Bowen Li, Fengze Pan, Haoyan Yin, Yanmin Gao and Feng Pan
Journal of power sources, Vol.653, p.237777
15/10/2025

Abstract

Chemistry Chemistry, Physical Electrochemistry Energy & Fuels Materials Science Materials Science, Multidisciplinary Physical Sciences Science & Technology Technology
We use modified carbon nanotubes (CNTs-COOC4H9) as a substrate to crystallize lithium iron phosphate on its surface in a non-uniform nucleation mode by controlling the nucleation driving force. Due to the presence of organic matter on the carbon nanotubes, a kind of "tree-root-like" electronic channels are formed inside the material after pyrolysis at high temperature, and these channels are connected by graphene oxide (GO), which dramatically enhances the electronic conductivity of the material. The prepared material achieves a reversible specific capacity of 168.2 mAh g-1 at 0.2C and a capacity retention of 97.7 % after 200 cycles. Even at high rates (2C, 5C, and 10C), they exhibit discharge specific capacities of 154.2, 135.8, and 114.1 mAh g-1 accordingly.
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https://doi.org/10.1016/j.jpowsour.2025.237777View
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